Symmetry studies in the nonlinear optical properties of molecular systems
J.L. Paz, L.G. Rodriguez, J.R. León-Torres, J.F. Cárdenas, L. Lascano, C. Costa-Vera
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Base Information
Volume
V49 - N4 / 2016 Ordinario
Reference
205-218
DOI
http://dx.doi.org/10.7149/OPA.49.4.49008
Language
Spanish
Keywords
Nonlinear optical properties, four-wave mixing, stochastic effects
Abstract
Symmetries of the nonlinear optical properties (rotation, reflection, inversion) of a two-level molecular system coupled to the thermal reservoir and interacting with classical electromagnetic fields, are studied. The thermal reservoir induces a time-dependent shift of the two-level resonance frequency. A perturbative methodology based in cumulant expansions to obtain the nonlinear macroscopic polarization, is employed. These symmetry properties show the dependence of the measured of the nonlinear optical properties with the variations in the frequencies of the incident fields.
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